We had similar issues when chrome archive could grow very large. This is our current config help reduce size dramatically.
[IncludeRegistryTrees]
HKCU\Software\Google\Chrome
[IncludeFolderTrees]
<LocalAppData>\Google\Chrome
[ExcludeFolderTrees]
<LocalAppData>\Google\Chrome\User Data\Default\Application Cache
<LocalAppData>\Google\Chrome\User Data\Default\Cache
<LocalAppData>\Google\Chrome\User Data\Default\Local Storage
<LocalAppData>\Google\Chrome\User Data\Default\Media Cache
<LocalAppData>\Google\Chrome\User Data\Default\Code Cache
<LocalAppData>\Google\Chrome\User Data\Default\Storage
<LocalAppData>\Google\Chrome\User Data\Default\GPUcache
<LocalAppData>\Google\Chrome\User Data\Default\Session Storage
<LocalAppData>\Google\Chrome\User Data\Default\Web Applications
<LocalAppData>\Google\Chrome\User Data\Default\Sync Data
<LocalAppData>\Google\Chrome\User Data\Default\Sync Data backup
<LocalAppData>\Google\Chrome\User Data\Default\Pepper Data\Shockwave Flash\CacheWriteableAdobeRoot
<LocalAppData>\Google\Chrome\User Data\Default\IndexedDB
<LocalAppData>\Google\Chrome\User Data\Profile 1\Cache
<LocalAppData>\Google\Chrome\User Data\Profile 1\Application Cache
<LocalAppData>\Google\Chrome\User Data\Profile 1\Storage
<LocalAppData>\Google\Chrome\User Data\Profile 1\Local Storage
<LocalAppData>\Google\Chrome\User Data\Profile 1\Media Cache
<LocalAppData>\Google\Chrome\User Data\Profile 1\Session Storage
<LocalAppData>\Google\Chrome\User Data\Profile 1\GPUCache
<LocalAppData>\Google\Chrome\User Data\Profile 1\Web Applications
<LocalAppData>\Google\Chrome\User Data\Profile 1\Sync Data
<LocalAppData>\Google\Chrome\User Data\Profile 1\Sync Data Backup
<LocalAppData>\Google\Chrome\User Data\Profile 1\Pepper Data\Shockwave Flash\CacheWriteableAdobeRoot
<LocalAppData>\Google\Chrome\User Data\Profile 1\IndexedDB
<LocalAppData>\Google\Chrome\User Data\Profile 2\Cache
<LocalAppData>\Google\Chrome\User Data\ShaderCache
<LocalAppData>\Google\Chrome\User Data\PepperFlash
<LocalAppData>\Google\Chrome\Application\
[ExcludeFiles]
<LocalAppData>\Google\Chrome\Default\Cache
<LocalAppData>\Google\Chrome\User Data\Default\ChromeDWriteFontCache
<LocalAppData>\Google\Chrome\User Data\Profile 1\ChromeDWriteFontCache
<LocalAppData>\Google\Chrome\User Data\Profile 2\ChromeDWriteFontCache
<LocalAppData>\Google\Chrome\User Data\Safe Browsing Bloom
<LocalAppData>\Google\Chrome\User Data\Safe Browsing Bloom Prefix Set
<LocalAppData>\Google\Chrome\User Data\Safe Browsing Download
<LocalAppData>\Google\Chrome\User Data\Safe Browsing UwS List
<LocalAppData>\Google\Chrome\User Data\Safe Browsing UwS List Prefix Set
<LocalAppData>\Google\Chrome\User Data\ev_hashes_whitelist.bin
*.tmp