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You can share the datastores between the clusters/vCenter without problem. And about the unregister/register task, just remember to shutdown the VM on old cluster before unregister from inventory.
Here is a blog post showing that you can shared datastore between clusters/vCenters: With vSphere 5.0 and HA can I share datastores across clusters?
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Richardson Porto
Senior Infrastructure Specialist
LinkedIn: http://linkedin.com/in/richardsonporto
Richardson Porto
Senior Infrastructure Specialist
LinkedIn: http://linkedin.com/in/richardsonporto